Targum for Genesis 4:6
וַיֹּ֥אמֶר יְהוָ֖ה אֶל־קָ֑יִן לָ֚מָּה חָ֣רָה לָ֔ךְ וְלָ֖מָּה נָפְל֥וּ פָנֶֽיךָ׃
And the LORD said unto Cain: ‘Why art thou wroth? and why is thy countenance fallen?
Targum Jonathan on Genesis
And the Lord said to Kain, Why hast thou anger, and why are the features of thy face downcast?
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